Thieno[3,2- b]thiophene-diketopyrrolopyrrole-containing polymers for high-performance organic field-effect transistors and organic photovoltaic devices

Hugo Bronstein; Zhuoying Chen; Raja Shahid Ashraf; Weimin Zhang; Junping Du; James R. Durrant; Pabitra Shakya Tuladhar; Kigook Song; Scott E. Watkins; Yves Geerts; Martijn M. Wienk; Rene A.J. Janssen; Thomas Anthopoulos; Henning Sirringhaus; Martin Heeney; Iain McCulloch

doi:10.1021/ja110619k

Thieno[3,2- b]thiophene-diketopyrrolopyrrole-containing polymers for high-performance organic field-effect transistors and organic photovoltaic devices

Hugo Bronstein^*, Zhuoying Chen, Raja Shahid Ashraf, Weimin Zhang, Junping Du, James R. Durrant, Pabitra Shakya Tuladhar, Kigook Song, Scott E. Watkins, Yves Geerts, Martijn M. Wienk, Rene A.J. Janssen, Thomas Anthopoulos, Henning Sirringhaus, Martin Heeney, Iain McCulloch

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

847 Scopus citations

Abstract

We report the synthesis and polymerization of a novel thieno[3,2-b] thiophene-diketopyrrolopyrrole-based monomer. Copolymerization with thiophene afforded a polymer with a maximum hole mobility of 1.95 cm² V ^-1 s^-1, which is the highest mobility from a polymer-based OFET reported to date. Bulk-heterojunction solar cells comprising this polymer and PC₇₁BM gave a power conversion efficiency of 5.4%.

Original language	English (US)
Pages (from-to)	3272-3275
Number of pages	4
Journal	Journal of the American Chemical Society
Volume	133
Issue number	10
DOIs	https://doi.org/10.1021/ja110619k
State	Published - Mar 16 2011
Externally published	Yes

Bibliographical note

Generated from Scopus record by KAUST IRTS on 2023-09-21

ASJC Scopus subject areas

General Chemistry
Biochemistry
Catalysis
Colloid and Surface Chemistry

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This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1021/ja110619k

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Bronstein, H., Chen, Z., Ashraf, R. S., Zhang, W., Du, J., Durrant, J. R., Shakya Tuladhar, P., Song, K., Watkins, S. E., Geerts, Y., Wienk, M. M., Janssen, R. A. J., Anthopoulos, T., Sirringhaus, H., Heeney, M., & McCulloch, I. (2011). Thieno[3,2- b]thiophene-diketopyrrolopyrrole-containing polymers for high-performance organic field-effect transistors and organic photovoltaic devices. Journal of the American Chemical Society, 133(10), 3272-3275. https://doi.org/10.1021/ja110619k

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title = "Thieno[3,2- b]thiophene-diketopyrrolopyrrole-containing polymers for high-performance organic field-effect transistors and organic photovoltaic devices",

abstract = "We report the synthesis and polymerization of a novel thieno[3,2-b] thiophene-diketopyrrolopyrrole-based monomer. Copolymerization with thiophene afforded a polymer with a maximum hole mobility of 1.95 cm2 V -1 s-1, which is the highest mobility from a polymer-based OFET reported to date. Bulk-heterojunction solar cells comprising this polymer and PC71BM gave a power conversion efficiency of 5.4%.",

author = "Hugo Bronstein and Zhuoying Chen and Ashraf, {Raja Shahid} and Weimin Zhang and Junping Du and Durrant, {James R.} and {Shakya Tuladhar}, Pabitra and Kigook Song and Watkins, {Scott E.} and Yves Geerts and Wienk, {Martijn M.} and Janssen, {Rene A.J.} and Thomas Anthopoulos and Henning Sirringhaus and Martin Heeney and Iain McCulloch",

note = "Generated from Scopus record by KAUST IRTS on 2023-09-21",

year = "2011",

month = mar,

day = "16",

doi = "10.1021/ja110619k",

language = "English (US)",

volume = "133",

pages = "3272--3275",

journal = "Journal of the American Chemical Society",

issn = "0002-7863",

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Bronstein, H, Chen, Z, Ashraf, RS, Zhang, W, Du, J, Durrant, JR, Shakya Tuladhar, P, Song, K, Watkins, SE, Geerts, Y, Wienk, MM, Janssen, RAJ, Anthopoulos, T, Sirringhaus, H, Heeney, M & McCulloch, I 2011, 'Thieno[3,2- b]thiophene-diketopyrrolopyrrole-containing polymers for high-performance organic field-effect transistors and organic photovoltaic devices', Journal of the American Chemical Society, vol. 133, no. 10, pp. 3272-3275. https://doi.org/10.1021/ja110619k

Thieno[3,2- b]thiophene-diketopyrrolopyrrole-containing polymers for high-performance organic field-effect transistors and organic photovoltaic devices. / Bronstein, Hugo; Chen, Zhuoying; Ashraf, Raja Shahid et al.
In: Journal of the American Chemical Society, Vol. 133, No. 10, 16.03.2011, p. 3272-3275.

Research output: Contribution to journal › Article › peer-review

TY - JOUR

T1 - Thieno[3,2- b]thiophene-diketopyrrolopyrrole-containing polymers for high-performance organic field-effect transistors and organic photovoltaic devices

AU - Bronstein, Hugo

AU - Chen, Zhuoying

AU - Ashraf, Raja Shahid

AU - Zhang, Weimin

AU - Du, Junping

AU - Durrant, James R.

AU - Shakya Tuladhar, Pabitra

AU - Song, Kigook

AU - Watkins, Scott E.

AU - Geerts, Yves

AU - Wienk, Martijn M.

AU - Janssen, Rene A.J.

AU - Anthopoulos, Thomas

AU - Sirringhaus, Henning

AU - Heeney, Martin

AU - McCulloch, Iain

N1 - Generated from Scopus record by KAUST IRTS on 2023-09-21

PY - 2011/3/16

Y1 - 2011/3/16

N2 - We report the synthesis and polymerization of a novel thieno[3,2-b] thiophene-diketopyrrolopyrrole-based monomer. Copolymerization with thiophene afforded a polymer with a maximum hole mobility of 1.95 cm2 V -1 s-1, which is the highest mobility from a polymer-based OFET reported to date. Bulk-heterojunction solar cells comprising this polymer and PC71BM gave a power conversion efficiency of 5.4%.

AB - We report the synthesis and polymerization of a novel thieno[3,2-b] thiophene-diketopyrrolopyrrole-based monomer. Copolymerization with thiophene afforded a polymer with a maximum hole mobility of 1.95 cm2 V -1 s-1, which is the highest mobility from a polymer-based OFET reported to date. Bulk-heterojunction solar cells comprising this polymer and PC71BM gave a power conversion efficiency of 5.4%.

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U2 - 10.1021/ja110619k

DO - 10.1021/ja110619k

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JF - Journal of the American Chemical Society

IS - 10

ER -

Thieno[3,2- b]thiophene-diketopyrrolopyrrole-containing polymers for high-performance organic field-effect transistors and organic photovoltaic devices

Abstract

Bibliographical note

ASJC Scopus subject areas

UN SDGs

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