The magnetic ordering in high magnetoresistance Mn-doped ZnO thin films

S. Venkatesh, Abdulaziz Mohammed Salem Ba Ras, J.-S. Lee, Iman S. Roqan

Research output: Contribution to journalArticlepeer-review

10 Scopus citations

Abstract

We studied the nature of magnetic ordering in Mn-doped ZnO thin films that exhibited ferromagnetism at 300 K and superparamagnetism at 5 K. We directly inter-related the magnetisation and magnetoresistance by invoking the polaronpercolation theory and variable range of hopping conduction below the metal-to-insulator transition. By obtaining a qualitative agreement between these two models, we attribute the ferromagnetism to the s-d exchange-induced spin splitting that was indicated by large positive magnetoresistance (∼40 %). Low temperature superparamagnetism was attributed to the localization of carriers and non-interacting polaron clusters. This analysis can assist in understanding the presence or absence of ferromagnetism in doped/un-doped ZnO.
Original languageEnglish (US)
Pages (from-to)035019
JournalAIP Advances
Volume6
Issue number3
DOIs
StatePublished - Mar 24 2016

Bibliographical note

KAUST Repository Item: Exported on 2020-10-01
Acknowledgements: The authors wish to thank KAUST for the financial support. Synchrotron studies were carried
out at the SSRL, a Directorate of SLAC and an Office of Science User Facility operated for the US DOE Office of Science by Stanford University. J.S.L. acknowledges partial funding from the
Global Research Laboratory program of the Korean Ministry of Education, Science, and Technology
(MEST). The authors also thank Dr. Paul R Edwards and Prof. Robert W Martin for using
EPMA facilities at University of Strathclyde.

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