Solvent-Solute Coordination Engineering for Efficient Perovskite Luminescent Solar Concentrators

Ziliang Li; Andrew Johnston; Mingyang Wei; Makhsud I. Saidaminov; Joao Martins de Pina; Xiaopeng Zheng; Jiakai Liu; Yuan Liu; Osman Bakr; Edward H. Sargent

doi:10.1016/j.joule.2020.01.003

Solvent-Solute Coordination Engineering for Efficient Perovskite Luminescent Solar Concentrators

Ziliang Li, Andrew Johnston, Mingyang Wei, Makhsud I. Saidaminov, Joao Martins de Pina, Xiaopeng Zheng, Jiakai Liu, Yuan Liu, Osman Bakr, Edward H. Sargent

Research output: Contribution to journal › Article › peer-review

67 Scopus citations

Abstract

By judiciously engineering solvent and anti-solvent ratios during the preparation of precursors, Li et al. exploit solvent-Pb2+ coordination to control the multiple quantum well (MQW) distribution in perovskite nanoplatelets (PNPLs). They report 10 × 10 cm luminescent solar concentrator (LSC) devices based on PNPL/poly(methyl methacrylate) composites; these reach an optical conversion efficiency of 2.0%.

Original language	English (US)
Journal	Joule
DOIs	https://doi.org/10.1016/j.joule.2020.01.003
State	Published - Feb 13 2020

Bibliographical note

KAUST Repository Item: Exported on 2020-10-01
Acknowledgements: This publication is based in part on work supported by the Ontario-Jiangsu Industrial R&D Program (OJIRDP). E.H.S. and all co-authors from the Department of Electrical and Computer Engineering at the University of Toronto acknowledge the financial support from the Ontario Research Fund−Research Excellence Program and the Natural Sciences and Engineering Research Council of Canada (NSERC). M.I.S. acknowledges the support of Banting Postdoctoral Fellowship Program, administered by the Government of Canada. X.Z. J.L. and O.M.B. acknowledge funding from King Abdullah University of Science and Technology (KAUST). GIWAXS measurements were performed at the HXMA beamline in the CLS, a national research facility of the University of Saskatchewan, which is supported by the Canada Foundation for Innovation (CFI), NSERC, the National Research Council (NRC), the Canadian Institutes of Health Research (CIHR), the Government of Saskatchewan, and the University of Saskatchewan. The authors acknowledge the technical assistance and scientific guidance of C.-Y. Kim at the CLS. Z.L. A.J. M.W. M.I.S. and E.H.S. conceived the idea and proposed the experimental design. Z.L. synthesized the materials and fabricated the devices. Z.L. J.M.P. and Y.L. performed the optical measurements. A.J. conducted the TA measurements. A.J. was responsible for the GIWAXS measurements. X.Z. J.L. and O.M.B. conducted the TEM measurements. Z.L. A.J. and E.H.S. co-wrote the manuscript. All authors contributed in data analysis and read and commented on the manuscript. The authors declare no competing interests.

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title = "Solvent-Solute Coordination Engineering for Efficient Perovskite Luminescent Solar Concentrators",

abstract = "By judiciously engineering solvent and anti-solvent ratios during the preparation of precursors, Li et al. exploit solvent-Pb2+ coordination to control the multiple quantum well (MQW) distribution in perovskite nanoplatelets (PNPLs). They report 10 × 10 cm luminescent solar concentrator (LSC) devices based on PNPL/poly(methyl methacrylate) composites; these reach an optical conversion efficiency of 2.0%.",

author = "Ziliang Li and Andrew Johnston and Mingyang Wei and Saidaminov, {Makhsud I.} and {Martins de Pina}, Joao and Xiaopeng Zheng and Jiakai Liu and Yuan Liu and Osman Bakr and Sargent, {Edward H.}",

note = "KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: This publication is based in part on work supported by the Ontario-Jiangsu Industrial R&D Program (OJIRDP). E.H.S. and all co-authors from the Department of Electrical and Computer Engineering at the University of Toronto acknowledge the financial support from the Ontario Research Fund−Research Excellence Program and the Natural Sciences and Engineering Research Council of Canada (NSERC). M.I.S. acknowledges the support of Banting Postdoctoral Fellowship Program, administered by the Government of Canada. X.Z. J.L. and O.M.B. acknowledge funding from King Abdullah University of Science and Technology (KAUST). GIWAXS measurements were performed at the HXMA beamline in the CLS, a national research facility of the University of Saskatchewan, which is supported by the Canada Foundation for Innovation (CFI), NSERC, the National Research Council (NRC), the Canadian Institutes of Health Research (CIHR), the Government of Saskatchewan, and the University of Saskatchewan. The authors acknowledge the technical assistance and scientific guidance of C.-Y. Kim at the CLS. Z.L. A.J. M.W. M.I.S. and E.H.S. conceived the idea and proposed the experimental design. Z.L. synthesized the materials and fabricated the devices. Z.L. J.M.P. and Y.L. performed the optical measurements. A.J. conducted the TA measurements. A.J. was responsible for the GIWAXS measurements. X.Z. J.L. and O.M.B. conducted the TEM measurements. Z.L. A.J. and E.H.S. co-wrote the manuscript. All authors contributed in data analysis and read and commented on the manuscript. The authors declare no competing interests.",

year = "2020",

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doi = "10.1016/j.joule.2020.01.003",

language = "English (US)",

journal = "Joule",

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AU - Li, Ziliang

AU - Johnston, Andrew

AU - Wei, Mingyang

AU - Saidaminov, Makhsud I.

AU - Martins de Pina, Joao

AU - Zheng, Xiaopeng

AU - Liu, Jiakai

AU - Liu, Yuan

AU - Bakr, Osman

AU - Sargent, Edward H.

N1 - KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: This publication is based in part on work supported by the Ontario-Jiangsu Industrial R&D Program (OJIRDP). E.H.S. and all co-authors from the Department of Electrical and Computer Engineering at the University of Toronto acknowledge the financial support from the Ontario Research Fund−Research Excellence Program and the Natural Sciences and Engineering Research Council of Canada (NSERC). M.I.S. acknowledges the support of Banting Postdoctoral Fellowship Program, administered by the Government of Canada. X.Z. J.L. and O.M.B. acknowledge funding from King Abdullah University of Science and Technology (KAUST). GIWAXS measurements were performed at the HXMA beamline in the CLS, a national research facility of the University of Saskatchewan, which is supported by the Canada Foundation for Innovation (CFI), NSERC, the National Research Council (NRC), the Canadian Institutes of Health Research (CIHR), the Government of Saskatchewan, and the University of Saskatchewan. The authors acknowledge the technical assistance and scientific guidance of C.-Y. Kim at the CLS. Z.L. A.J. M.W. M.I.S. and E.H.S. conceived the idea and proposed the experimental design. Z.L. synthesized the materials and fabricated the devices. Z.L. J.M.P. and Y.L. performed the optical measurements. A.J. conducted the TA measurements. A.J. was responsible for the GIWAXS measurements. X.Z. J.L. and O.M.B. conducted the TEM measurements. Z.L. A.J. and E.H.S. co-wrote the manuscript. All authors contributed in data analysis and read and commented on the manuscript. The authors declare no competing interests.

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N2 - By judiciously engineering solvent and anti-solvent ratios during the preparation of precursors, Li et al. exploit solvent-Pb2+ coordination to control the multiple quantum well (MQW) distribution in perovskite nanoplatelets (PNPLs). They report 10 × 10 cm luminescent solar concentrator (LSC) devices based on PNPL/poly(methyl methacrylate) composites; these reach an optical conversion efficiency of 2.0%.

AB - By judiciously engineering solvent and anti-solvent ratios during the preparation of precursors, Li et al. exploit solvent-Pb2+ coordination to control the multiple quantum well (MQW) distribution in perovskite nanoplatelets (PNPLs). They report 10 × 10 cm luminescent solar concentrator (LSC) devices based on PNPL/poly(methyl methacrylate) composites; these reach an optical conversion efficiency of 2.0%.

UR - http://hdl.handle.net/10754/661582

UR - https://linkinghub.elsevier.com/retrieve/pii/S2542435120300301

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JO - Joule

JF - Joule

ER -

Solvent-Solute Coordination Engineering for Efficient Perovskite Luminescent Solar Concentrators

Abstract

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