Solution-Processed Mixed-Dimensional Hybrid Perovskite/Carbon Nanotube Electronics.

Chun Ma; Sarah Clark; Zhixiong Liu; Liangliang Liang; Yuliar Firdaus; Ran Tao; Ali Han; Xiaogang Liu; Lain-Jong Li; Thomas D. Anthopoulos; Mark C Hersam; Tao Wu

doi:10.1021/acsnano.9b07888

Solution-Processed Mixed-Dimensional Hybrid Perovskite/Carbon Nanotube Electronics.

Chun Ma, Sarah Clark, Zhixiong Liu, Liangliang Liang, Yuliar Firdaus, Ran Tao, Ali Han, Xiaogang Liu, Lain-Jong Li, Thomas D. Anthopoulos, Mark C Hersam, Tao Wu

Research output: Contribution to journal › Article › peer-review

30 Scopus citations

Abstract

Benefiting from their extraordinary physical properties, methylammonium lead halide perovskites (PVKs) have attracted significant attention in optoelectronics. However, the PVK-based devices suffer from low carrier mobility and high operation voltage. Here, we utilize sorted semiconducting single-walled carbon nanotubes (95% s-SWCNTs) to enhance the performance of thin-film transistors (TFTs) based on the mixed-cation perovskite (MA1-xFAx)Pb(I1-xBrx)3, enabling mixed-dimensional solution-processed electronics with high mobility (32.25 cm2/(V s)) and low voltage (∼3 V) operation. The resulting mixed-dimensional PVK/SWCNT TFTs possess ON/OFF ratios on the order of 107, enabling the fabrication of high-gain inverters.

Original language	English (US)
Pages (from-to)	3969-3979
Number of pages	11
Journal	ACS nano
Volume	14
Issue number	4
DOIs	https://doi.org/10.1021/acsnano.9b07888
State	Published - Mar 3 2020

Bibliographical note

KAUST Repository Item: Exported on 2020-10-01
Acknowledgements: This research was supported by the Materials Research Science and Engineering Center (MRSEC) of Northwestern University (NSFDMR-1720139). This research was supported by Material Science and Engineering (MSE) of King Abdullah University of Science and Technology. T.W. and M.H. conceived and supervised the project. C.M., S.C., L.L., R.T., and A.H. wrote the paper. C.M., Z.L., and A.H. fabricated and characterized the devices. Y.F. performed ellipsometry. S.C. synthesized unsorted and sorted s-SWCNT. L.J.L. provided
metallic SWCNTs. All authors discussed the results

Access to Document

10.1021/acsnano.9b07888

https://repository.kaust.edu.sa/bitstream/10754/662383/1/Chun%20Deposit.pdf

Cite this

@article{595c8db5581d427d946e789dce05f72e,

title = "Solution-Processed Mixed-Dimensional Hybrid Perovskite/Carbon Nanotube Electronics.",

abstract = "Benefiting from their extraordinary physical properties, methylammonium lead halide perovskites (PVKs) have attracted significant attention in optoelectronics. However, the PVK-based devices suffer from low carrier mobility and high operation voltage. Here, we utilize sorted semiconducting single-walled carbon nanotubes (95% s-SWCNTs) to enhance the performance of thin-film transistors (TFTs) based on the mixed-cation perovskite (MA1-xFAx)Pb(I1-xBrx)3, enabling mixed-dimensional solution-processed electronics with high mobility (32.25 cm2/(V s)) and low voltage (∼3 V) operation. The resulting mixed-dimensional PVK/SWCNT TFTs possess ON/OFF ratios on the order of 107, enabling the fabrication of high-gain inverters.",

author = "Chun Ma and Sarah Clark and Zhixiong Liu and Liangliang Liang and Yuliar Firdaus and Ran Tao and Ali Han and Xiaogang Liu and Lain-Jong Li and Anthopoulos, {Thomas D.} and Hersam, {Mark C} and Tao Wu",

note = "KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: This research was supported by the Materials Research Science and Engineering Center (MRSEC) of Northwestern University (NSFDMR-1720139). This research was supported by Material Science and Engineering (MSE) of King Abdullah University of Science and Technology. T.W. and M.H. conceived and supervised the project. C.M., S.C., L.L., R.T., and A.H. wrote the paper. C.M., Z.L., and A.H. fabricated and characterized the devices. Y.F. performed ellipsometry. S.C. synthesized unsorted and sorted s-SWCNT. L.J.L. provided metallic SWCNTs. All authors discussed the results",

year = "2020",

month = mar,

day = "3",

doi = "10.1021/acsnano.9b07888",

language = "English (US)",

volume = "14",

pages = "3969--3979",

journal = "ACS nano",

issn = "1936-0851",

publisher = "American Chemical Society",

number = "4",

}

TY - JOUR

T1 - Solution-Processed Mixed-Dimensional Hybrid Perovskite/Carbon Nanotube Electronics.

AU - Ma, Chun

AU - Clark, Sarah

AU - Liu, Zhixiong

AU - Liang, Liangliang

AU - Firdaus, Yuliar

AU - Tao, Ran

AU - Han, Ali

AU - Liu, Xiaogang

AU - Li, Lain-Jong

AU - Anthopoulos, Thomas D.

AU - Hersam, Mark C

AU - Wu, Tao

N1 - KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: This research was supported by the Materials Research Science and Engineering Center (MRSEC) of Northwestern University (NSFDMR-1720139). This research was supported by Material Science and Engineering (MSE) of King Abdullah University of Science and Technology. T.W. and M.H. conceived and supervised the project. C.M., S.C., L.L., R.T., and A.H. wrote the paper. C.M., Z.L., and A.H. fabricated and characterized the devices. Y.F. performed ellipsometry. S.C. synthesized unsorted and sorted s-SWCNT. L.J.L. provided metallic SWCNTs. All authors discussed the results

PY - 2020/3/3

Y1 - 2020/3/3

N2 - Benefiting from their extraordinary physical properties, methylammonium lead halide perovskites (PVKs) have attracted significant attention in optoelectronics. However, the PVK-based devices suffer from low carrier mobility and high operation voltage. Here, we utilize sorted semiconducting single-walled carbon nanotubes (95% s-SWCNTs) to enhance the performance of thin-film transistors (TFTs) based on the mixed-cation perovskite (MA1-xFAx)Pb(I1-xBrx)3, enabling mixed-dimensional solution-processed electronics with high mobility (32.25 cm2/(V s)) and low voltage (∼3 V) operation. The resulting mixed-dimensional PVK/SWCNT TFTs possess ON/OFF ratios on the order of 107, enabling the fabrication of high-gain inverters.

AB - Benefiting from their extraordinary physical properties, methylammonium lead halide perovskites (PVKs) have attracted significant attention in optoelectronics. However, the PVK-based devices suffer from low carrier mobility and high operation voltage. Here, we utilize sorted semiconducting single-walled carbon nanotubes (95% s-SWCNTs) to enhance the performance of thin-film transistors (TFTs) based on the mixed-cation perovskite (MA1-xFAx)Pb(I1-xBrx)3, enabling mixed-dimensional solution-processed electronics with high mobility (32.25 cm2/(V s)) and low voltage (∼3 V) operation. The resulting mixed-dimensional PVK/SWCNT TFTs possess ON/OFF ratios on the order of 107, enabling the fabrication of high-gain inverters.

UR - http://hdl.handle.net/10754/662383

UR - https://pubs.acs.org/doi/10.1021/acsnano.9b07888

UR - http://www.scopus.com/inward/record.url?scp=85084167664&partnerID=8YFLogxK

U2 - 10.1021/acsnano.9b07888

DO - 10.1021/acsnano.9b07888

M3 - Article

C2 - 32119769

SN - 1936-0851

VL - 14

SP - 3969

EP - 3979

JO - ACS nano

JF - ACS nano

IS - 4

ER -

Solution-Processed Mixed-Dimensional Hybrid Perovskite/Carbon Nanotube Electronics.

Abstract

Bibliographical note

Access to Document

Other files and links

Fingerprint

Cite this