Single-atom nickel terminating sp2 and sp3 nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting

Yanrui Li; Yiqing Wang; Chung-Li Dong; Yu-Cheng Huang; Jie Chen; Zhen Zhang; Fanqi Meng; Qinghua Zhang; Yiliang Huangfu; Daming Zhao; Lin Gu; Shaohua Shen

doi:10.1039/d0sc07093a

Single-atom nickel terminating sp2 and sp3 nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting

Yanrui Li, Yiqing Wang, Chung-Li Dong, Yu-Cheng Huang, Jie Chen, Zhen Zhang, Fanqi Meng, Qinghua Zhang, Yiliang Huangfu, Daming Zhao, Lin Gu, Shaohua Shen

King Abdullah University of Science and Technology

Research output: Contribution to journal › Article › peer-review

87 Scopus citations

Abstract

Single-atom Ni terminating agent is introduced to coordinate with sp$^{2}$ or sp$^{3}$ N atoms in the heptazine units of PCN, realizing visible-light photocatalytic overall water splitting to H$_{2}$O$_{2}$ and H$_{2}$ without additional cocatalyst.

Original language	English (US)
Journal	Chemical Science
DOIs	https://doi.org/10.1039/d0sc07093a
State	Published - 2021

Bibliographical note

KAUST Repository Item: Exported on 2021-02-08
Acknowledgements: This work was supported by the National Natural Science Foundation of China (51961165103 and 21875183), the National Key Research and Development Program of China (2017YFE0193900), the National Program for Support of Top notch Young Professionals, the “Fundamental Research Funds for the Central Universities”, the Project Supported by the Natural Science Basic Research Plan in Shaanxi Province of
China (2018JQ2028), the China Postdoctoral Science Foundation (2018M640981), and “The Youth Innovation Team of Shaanxi Universities”. C.L.D is grateful to MoST for financially supporting this work under contracts MoST 107-2112-M-032-004-MY3 and 108-2218-E-032-003-MY3.

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10.1039/d0sc07093a

https://repository.kaust.edu.sa/bitstream/10754/667244/1/single%20atom.pdf

Cite this

@article{51a3494bf6b14ca6ab29e5aac8ff053d,

title = "Single-atom nickel terminating sp2 and sp3 nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting",

abstract = "Single-atom Ni terminating agent is introduced to coordinate with sp$^{2}$ or sp$^{3}$ N atoms in the heptazine units of PCN, realizing visible-light photocatalytic overall water splitting to H$_{2}$O$_{2}$ and H$_{2}$ without additional cocatalyst.",

author = "Yanrui Li and Yiqing Wang and Chung-Li Dong and Yu-Cheng Huang and Jie Chen and Zhen Zhang and Fanqi Meng and Qinghua Zhang and Yiliang Huangfu and Daming Zhao and Lin Gu and Shaohua Shen",

note = "KAUST Repository Item: Exported on 2021-02-08 Acknowledgements: This work was supported by the National Natural Science Foundation of China (51961165103 and 21875183), the National Key Research and Development Program of China (2017YFE0193900), the National Program for Support of Top notch Young Professionals, the “Fundamental Research Funds for the Central Universities”, the Project Supported by the Natural Science Basic Research Plan in Shaanxi Province of China (2018JQ2028), the China Postdoctoral Science Foundation (2018M640981), and “The Youth Innovation Team of Shaanxi Universities”. C.L.D is grateful to MoST for financially supporting this work under contracts MoST 107-2112-M-032-004-MY3 and 108-2218-E-032-003-MY3.",

year = "2021",

doi = "10.1039/d0sc07093a",

language = "English (US)",

journal = "Chemical Science",

issn = "2041-6520",

publisher = "Royal Society of Chemistry",

}

TY - JOUR

T1 - Single-atom nickel terminating sp2 and sp3 nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting

AU - Li, Yanrui

AU - Wang, Yiqing

AU - Dong, Chung-Li

AU - Huang, Yu-Cheng

AU - Chen, Jie

AU - Zhang, Zhen

AU - Meng, Fanqi

AU - Zhang, Qinghua

AU - Huangfu, Yiliang

AU - Zhao, Daming

AU - Gu, Lin

AU - Shen, Shaohua

N1 - KAUST Repository Item: Exported on 2021-02-08 Acknowledgements: This work was supported by the National Natural Science Foundation of China (51961165103 and 21875183), the National Key Research and Development Program of China (2017YFE0193900), the National Program for Support of Top notch Young Professionals, the “Fundamental Research Funds for the Central Universities”, the Project Supported by the Natural Science Basic Research Plan in Shaanxi Province of China (2018JQ2028), the China Postdoctoral Science Foundation (2018M640981), and “The Youth Innovation Team of Shaanxi Universities”. C.L.D is grateful to MoST for financially supporting this work under contracts MoST 107-2112-M-032-004-MY3 and 108-2218-E-032-003-MY3.

PY - 2021

Y1 - 2021

N2 - Single-atom Ni terminating agent is introduced to coordinate with sp$^{2}$ or sp$^{3}$ N atoms in the heptazine units of PCN, realizing visible-light photocatalytic overall water splitting to H$_{2}$O$_{2}$ and H$_{2}$ without additional cocatalyst.

AB - Single-atom Ni terminating agent is introduced to coordinate with sp$^{2}$ or sp$^{3}$ N atoms in the heptazine units of PCN, realizing visible-light photocatalytic overall water splitting to H$_{2}$O$_{2}$ and H$_{2}$ without additional cocatalyst.

UR - http://hdl.handle.net/10754/667244

UR - http://xlink.rsc.org/?DOI=D0SC07093A

U2 - 10.1039/d0sc07093a

DO - 10.1039/d0sc07093a

M3 - Article

C2 - 34163637

SN - 2041-6520

JO - Chemical Science

JF - Chemical Science

ER -

Single-atom nickel terminating sp2 and sp3 nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting

Abstract

Bibliographical note

UN SDGs

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