Single-atom nickel terminating sp2 and sp3 nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting

Yanrui Li, Yiqing Wang, Chung-Li Dong, Yu-Cheng Huang, Jie Chen, Zhen Zhang, Fanqi Meng, Qinghua Zhang, Yiliang Huangfu, Daming Zhao, Lin Gu, Shaohua Shen

Research output: Contribution to journalArticlepeer-review

69 Scopus citations

Abstract

Single-atom Ni terminating agent is introduced to coordinate with sp$^{2}$ or sp$^{3}$ N atoms in the heptazine units of PCN, realizing visible-light photocatalytic overall water splitting to H$_{2}$O$_{2}$ and H$_{2}$ without additional cocatalyst.
Original languageEnglish (US)
JournalChemical Science
DOIs
StatePublished - 2021

Bibliographical note

KAUST Repository Item: Exported on 2021-02-08
Acknowledgements: This work was supported by the National Natural Science Foundation of China (51961165103 and 21875183), the National Key Research and Development Program of China (2017YFE0193900), the National Program for Support of Top notch Young Professionals, the “Fundamental Research Funds for the Central Universities”, the Project Supported by the Natural Science Basic Research Plan in Shaanxi Province of
China (2018JQ2028), the China Postdoctoral Science Foundation (2018M640981), and “The Youth Innovation Team of Shaanxi Universities”. C.L.D is grateful to MoST for financially supporting this work under contracts MoST 107-2112-M-032-004-MY3 and 108-2218-E-032-003-MY3.

Fingerprint

Dive into the research topics of 'Single-atom nickel terminating sp2 and sp3 nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting'. Together they form a unique fingerprint.

Cite this