Revealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling

Seungtaik Hwang; Rocio Semino; Beatriz Seoane; Marufa Zahan; Christian Chmelik; Rustem Valiullin; Marko Bertmer; Jürgen Haase; Freek Kapteijn; Jorge Gascon; Guillaume Maurin; Jörg Kärger

doi:10.1002/anie.201713160

Revealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling

Seungtaik Hwang, Rocio Semino, Beatriz Seoane, Marufa Zahan, Christian Chmelik, Rustem Valiullin, Marko Bertmer, Jürgen Haase, Freek Kapteijn, Jorge Gascon, Guillaume Maurin, Jörg Kärger

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Abstract

Through IR microimaging the spatially and temporally resolved development of the CO2 concentration in a ZIF-8@6FDA-DAM mixed matrix membrane was visualized during transient adsorption. By recording the evolution of the CO2 concentration, it is observed that the CO2 molecules propagate from the ZIF-8 filler, which acts as a transport

Original language	English (US)
Pages (from-to)	5156-5160
Number of pages	5
Journal	Angewandte Chemie International Edition
Volume	57
Issue number	18
DOIs	https://doi.org/10.1002/anie.201713160 https://doi.org/10.1002/ange.201713160
State	Published - Mar 25 2018

Bibliographical note

KAUST Repository Item: Exported on 2020-10-01
Acknowledgements: The research leading to these results has received funding from the European Community Seventh Program (FP7/2007-2013) under Grant 608490 (project M4CO2). IR microimaging was ensured by German Science Foundation via the grants HA 1893/17-1 and KA 953/35-1. G.M. thanks Institut Universitaire de France for its support. The authors thank J. Caro (Hannover) for stimulating discussions and synthesizing the large ZIF-8 crystals.

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https://repository.kaust.edu.sa/bitstream/10754/627202/1/Hwang_et_al-2018-Angewandte_Chemie_International_Edition.pdf

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Hwang, S., Semino, R., Seoane, B., Zahan, M., Chmelik, C., Valiullin, R., Bertmer, M., Haase, J., Kapteijn, F., Gascon, J., Maurin, G., & Kärger, J. (2018). Revealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling. Angewandte Chemie International Edition, 57(18), 5156-5160. https://doi.org/10.1002/anie.201713160, https://doi.org/10.1002/ange.201713160

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title = "Revealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling",

abstract = "Through IR microimaging the spatially and temporally resolved development of the CO2 concentration in a ZIF-8@6FDA-DAM mixed matrix membrane was visualized during transient adsorption. By recording the evolution of the CO2 concentration, it is observed that the CO2 molecules propagate from the ZIF-8 filler, which acts as a transport",

author = "Seungtaik Hwang and Rocio Semino and Beatriz Seoane and Marufa Zahan and Christian Chmelik and Rustem Valiullin and Marko Bertmer and J{\"u}rgen Haase and Freek Kapteijn and Jorge Gascon and Guillaume Maurin and J{\"o}rg K{\"a}rger",

note = "KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: The research leading to these results has received funding from the European Community Seventh Program (FP7/2007-2013) under Grant 608490 (project M4CO2). IR microimaging was ensured by German Science Foundation via the grants HA 1893/17-1 and KA 953/35-1. G.M. thanks Institut Universitaire de France for its support. The authors thank J. Caro (Hannover) for stimulating discussions and synthesizing the large ZIF-8 crystals.",

year = "2018",

month = mar,

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doi = "10.1002/anie.201713160",

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journal = "Angewandte Chemie International Edition",

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Hwang, S, Semino, R, Seoane, B, Zahan, M, Chmelik, C, Valiullin, R, Bertmer, M, Haase, J, Kapteijn, F, Gascon, J, Maurin, G & Kärger, J 2018, 'Revealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling', Angewandte Chemie International Edition, vol. 57, no. 18, pp. 5156-5160. https://doi.org/10.1002/anie.201713160, https://doi.org/10.1002/ange.201713160

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T1 - Revealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling

AU - Hwang, Seungtaik

AU - Semino, Rocio

AU - Seoane, Beatriz

AU - Zahan, Marufa

AU - Chmelik, Christian

AU - Valiullin, Rustem

AU - Bertmer, Marko

AU - Haase, Jürgen

AU - Kapteijn, Freek

AU - Gascon, Jorge

AU - Maurin, Guillaume

AU - Kärger, Jörg

N1 - KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: The research leading to these results has received funding from the European Community Seventh Program (FP7/2007-2013) under Grant 608490 (project M4CO2). IR microimaging was ensured by German Science Foundation via the grants HA 1893/17-1 and KA 953/35-1. G.M. thanks Institut Universitaire de France for its support. The authors thank J. Caro (Hannover) for stimulating discussions and synthesizing the large ZIF-8 crystals.

PY - 2018/3/25

Y1 - 2018/3/25

N2 - Through IR microimaging the spatially and temporally resolved development of the CO2 concentration in a ZIF-8@6FDA-DAM mixed matrix membrane was visualized during transient adsorption. By recording the evolution of the CO2 concentration, it is observed that the CO2 molecules propagate from the ZIF-8 filler, which acts as a transport

AB - Through IR microimaging the spatially and temporally resolved development of the CO2 concentration in a ZIF-8@6FDA-DAM mixed matrix membrane was visualized during transient adsorption. By recording the evolution of the CO2 concentration, it is observed that the CO2 molecules propagate from the ZIF-8 filler, which acts as a transport

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ER -

Revealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling

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