In situ real-time monitoring of Pt-VO2 nanoparticle-nanowire assembly by GISAXS

Cafer T. Yavuz; Sungsik Lee; Byeongdu Lee; Myung H. Kim; Jeong M. Baik; Sönke Seifert; Stefan Vajda; Christopher Larson; Randall E. Winans; Martin Moskovits; Alec M. Wodtke; Galen D. Stucky

doi:10.1117/12.851255

In situ real-time monitoring of Pt-VO2 nanoparticle-nanowire assembly by GISAXS

Cafer T. Yavuz, Sungsik Lee, Byeongdu Lee, Myung H. Kim, Jeong M. Baik, Sönke Seifert, Stefan Vajda, Christopher Larson, Randall E. Winans, Martin Moskovits, Alec M. Wodtke, Galen D. Stucky

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

3 Scopus citations

Abstract

Methanol is a hydrogen carrier for fuel cells and its chemical transformations are of great current interest. Methanol oxidation by vanadium oxides is well studied, hence, serves as a good measure for catalytic activity. Arrays of VO2 nanowires grown on r-cut sapphire prove to be unique for the in situ catalytic activity tests. Here, we present size and morphology dependent activity of Platinum coated single crystalline VO2 nanowires in methanol oxidation reactions using Grazing Incidence Small Angle X-ray Scattering (GISAXS). Our findings show an unexpected sintering behavior of Pt at temperatures as low as 200 °C. © 2010 Copyright SPIE - The International Society for Optical Engineering.

Original language	English (US)
Title of host publication	Proceedings of SPIE - The International Society for Optical Engineering
DOIs	https://doi.org/10.1117/12.851255
State	Published - Dec 1 2010
Externally published	Yes

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title = "In situ real-time monitoring of Pt-VO2 nanoparticle-nanowire assembly by GISAXS",

abstract = "Methanol is a hydrogen carrier for fuel cells and its chemical transformations are of great current interest. Methanol oxidation by vanadium oxides is well studied, hence, serves as a good measure for catalytic activity. Arrays of VO2 nanowires grown on r-cut sapphire prove to be unique for the in situ catalytic activity tests. Here, we present size and morphology dependent activity of Platinum coated single crystalline VO2 nanowires in methanol oxidation reactions using Grazing Incidence Small Angle X-ray Scattering (GISAXS). Our findings show an unexpected sintering behavior of Pt at temperatures as low as 200 °C. {\textcopyright} 2010 Copyright SPIE - The International Society for Optical Engineering.",

author = "Yavuz, {Cafer T.} and Sungsik Lee and Byeongdu Lee and Kim, {Myung H.} and Baik, {Jeong M.} and S{\"o}nke Seifert and Stefan Vajda and Christopher Larson and Winans, {Randall E.} and Martin Moskovits and Wodtke, {Alec M.} and Stucky, {Galen D.}",

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year = "2010",

month = dec,

day = "1",

doi = "10.1117/12.851255",

language = "English (US)",

isbn = "9780819481436",

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T1 - In situ real-time monitoring of Pt-VO2 nanoparticle-nanowire assembly by GISAXS

AU - Yavuz, Cafer T.

AU - Lee, Sungsik

AU - Lee, Byeongdu

AU - Kim, Myung H.

AU - Baik, Jeong M.

AU - Seifert, Sönke

AU - Vajda, Stefan

AU - Larson, Christopher

AU - Winans, Randall E.

AU - Moskovits, Martin

AU - Wodtke, Alec M.

AU - Stucky, Galen D.

N1 - Generated from Scopus record by KAUST IRTS on 2021-03-16

PY - 2010/12/1

Y1 - 2010/12/1

N2 - Methanol is a hydrogen carrier for fuel cells and its chemical transformations are of great current interest. Methanol oxidation by vanadium oxides is well studied, hence, serves as a good measure for catalytic activity. Arrays of VO2 nanowires grown on r-cut sapphire prove to be unique for the in situ catalytic activity tests. Here, we present size and morphology dependent activity of Platinum coated single crystalline VO2 nanowires in methanol oxidation reactions using Grazing Incidence Small Angle X-ray Scattering (GISAXS). Our findings show an unexpected sintering behavior of Pt at temperatures as low as 200 °C. © 2010 Copyright SPIE - The International Society for Optical Engineering.

AB - Methanol is a hydrogen carrier for fuel cells and its chemical transformations are of great current interest. Methanol oxidation by vanadium oxides is well studied, hence, serves as a good measure for catalytic activity. Arrays of VO2 nanowires grown on r-cut sapphire prove to be unique for the in situ catalytic activity tests. Here, we present size and morphology dependent activity of Platinum coated single crystalline VO2 nanowires in methanol oxidation reactions using Grazing Incidence Small Angle X-ray Scattering (GISAXS). Our findings show an unexpected sintering behavior of Pt at temperatures as low as 200 °C. © 2010 Copyright SPIE - The International Society for Optical Engineering.

UR - http://proceedings.spiedigitallibrary.org/proceeding.aspx?doi=10.1117/12.851255

UR - http://www.scopus.com/inward/record.url?scp=79953763902&partnerID=8YFLogxK

U2 - 10.1117/12.851255

DO - 10.1117/12.851255

M3 - Conference contribution

SN - 9780819481436

BT - Proceedings of SPIE - The International Society for Optical Engineering

ER -

In situ real-time monitoring of Pt-VO2 nanoparticle-nanowire assembly by GISAXS

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