Highly efficient perovskite solar cells with crosslinked PCBM interlayers

W. Qiu; J. P. Bastos; S. Dasgupta; T. Merckx; I. Cardinaletti; M. V. C. Jenart; C. B. Nielsen; R. Gehlhaar; J. Poortmans; P. Heremans; Iain McCulloch; D. Cheyns

doi:10.1039/c6ta08799j

Highly efficient perovskite solar cells with crosslinked PCBM interlayers

W. Qiu, J. P. Bastos, S. Dasgupta, T. Merckx, I. Cardinaletti, M. V. C. Jenart, C. B. Nielsen, R. Gehlhaar, J. Poortmans, P. Heremans, Iain McCulloch, D. Cheyns

Research output: Contribution to journal › Article › peer-review

54 Scopus citations

Abstract

Commercially available phenyl-C-butyric acid methyl ester (PCBM) is crosslinked with 1,6-diazidohexane (DAZH), resulting in films resistant to common solvents used in perovskite solar cell processing. By using crosslinked PCBM as an interlayer and (HC(NH))(CHNH)PbIBr as the active layer, we achieve small area devices and modules with a maximum steady-state power conversion efficiency of 18.1% and 14.9%, respectively.

Original language	English (US)
Pages (from-to)	2466-2472
Number of pages	7
Journal	J. Mater. Chem. A
Volume	5
Issue number	6
DOIs	https://doi.org/10.1039/c6ta08799j
State	Published - 2017

Bibliographical note

KAUST Repository Item: Exported on 2020-10-01
Acknowledgements: W. Qiu would like to acknowledge Ziyang Liu for taking the SEM images. This research has received (partial) funding from the Flemish Government – Department of Economics, Science and Innovation. This work has been partially supported by Solliance, a partnership of R&D organizations from Belgium, the Netherlands, and Germany working in thin film photovoltaic solar energy.

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title = "Highly efficient perovskite solar cells with crosslinked PCBM interlayers",

abstract = "Commercially available phenyl-C-butyric acid methyl ester (PCBM) is crosslinked with 1,6-diazidohexane (DAZH), resulting in films resistant to common solvents used in perovskite solar cell processing. By using crosslinked PCBM as an interlayer and (HC(NH))(CHNH)PbIBr as the active layer, we achieve small area devices and modules with a maximum steady-state power conversion efficiency of 18.1% and 14.9%, respectively.",

author = "W. Qiu and Bastos, {J. P.} and S. Dasgupta and T. Merckx and I. Cardinaletti and Jenart, {M. V. C.} and Nielsen, {C. B.} and R. Gehlhaar and J. Poortmans and P. Heremans and Iain McCulloch and D. Cheyns",

note = "KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: W. Qiu would like to acknowledge Ziyang Liu for taking the SEM images. This research has received (partial) funding from the Flemish Government – Department of Economics, Science and Innovation. This work has been partially supported by Solliance, a partnership of R&D organizations from Belgium, the Netherlands, and Germany working in thin film photovoltaic solar energy.",

year = "2017",

doi = "10.1039/c6ta08799j",

language = "English (US)",

volume = "5",

pages = "2466--2472",

journal = "J. Mater. Chem. A",

issn = "2050-7488",

publisher = "Royal Society of Chemistry",

number = "6",

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TY - JOUR

T1 - Highly efficient perovskite solar cells with crosslinked PCBM interlayers

AU - Qiu, W.

AU - Bastos, J. P.

AU - Dasgupta, S.

AU - Merckx, T.

AU - Cardinaletti, I.

AU - Jenart, M. V. C.

AU - Nielsen, C. B.

AU - Gehlhaar, R.

AU - Poortmans, J.

AU - Heremans, P.

AU - McCulloch, Iain

AU - Cheyns, D.

N1 - KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: W. Qiu would like to acknowledge Ziyang Liu for taking the SEM images. This research has received (partial) funding from the Flemish Government – Department of Economics, Science and Innovation. This work has been partially supported by Solliance, a partnership of R&D organizations from Belgium, the Netherlands, and Germany working in thin film photovoltaic solar energy.

PY - 2017

Y1 - 2017

N2 - Commercially available phenyl-C-butyric acid methyl ester (PCBM) is crosslinked with 1,6-diazidohexane (DAZH), resulting in films resistant to common solvents used in perovskite solar cell processing. By using crosslinked PCBM as an interlayer and (HC(NH))(CHNH)PbIBr as the active layer, we achieve small area devices and modules with a maximum steady-state power conversion efficiency of 18.1% and 14.9%, respectively.

AB - Commercially available phenyl-C-butyric acid methyl ester (PCBM) is crosslinked with 1,6-diazidohexane (DAZH), resulting in films resistant to common solvents used in perovskite solar cell processing. By using crosslinked PCBM as an interlayer and (HC(NH))(CHNH)PbIBr as the active layer, we achieve small area devices and modules with a maximum steady-state power conversion efficiency of 18.1% and 14.9%, respectively.

UR - http://hdl.handle.net/10754/623842

UR - http://pubs.rsc.org/en/Content/ArticleLanding/2017/TA/C6TA08799J#!divAbstract

UR - http://www.scopus.com/inward/record.url?scp=85012028853&partnerID=8YFLogxK

U2 - 10.1039/c6ta08799j

DO - 10.1039/c6ta08799j

M3 - Article

SN - 2050-7488

VL - 5

SP - 2466

EP - 2472

JO - J. Mater. Chem. A

JF - J. Mater. Chem. A

IS - 6

ER -

Highly efficient perovskite solar cells with crosslinked PCBM interlayers

Abstract

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