Highly Efficient Perovskite-Quantum-Dot Light-Emitting Diodes by Surface Engineering

Jun Pan; Li Na Quan; Yongbiao Zhao; Wei Peng; Murali Banavoth; Smritakshi P. Sarmah; Mingjian Yuan; Lutfan Sinatra; Noktan Mohammed AlYami; Jiakai Liu; Emre Yassitepe; Zhenyu Yang; Oleksandr Voznyy; Riccardo Comin; Mohamed N. Hedhili; Omar F. Mohammed; Zheng Hong Lu; Dong Ha Kim; Edward H. Sargent; Osman Bakr

doi:10.1002/adma.201600784

Highly Efficient Perovskite-Quantum-Dot Light-Emitting Diodes by Surface Engineering

Jun Pan, Li Na Quan, Yongbiao Zhao, Wei Peng, Murali Banavoth, Smritakshi P. Sarmah, Mingjian Yuan, Lutfan Sinatra, Noktan Mohammed AlYami, Jiakai Liu, Emre Yassitepe, Zhenyu Yang, Oleksandr Voznyy, Riccardo Comin, Mohamed N. Hedhili, Omar F. Mohammed, Zheng Hong Lu, Dong Ha Kim, Edward H. Sargent, Osman Bakr

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985 Scopus citations

Abstract

A two-step ligand-exchange strategy is developed, in which the long-carbon-chain ligands on all-inorganic perovskite (CsPbX3, X = Br, Cl) quantum dots (QDs) are replaced with halide-ion-pair ligands. Green and blue light-emitting diodes made from the halide-ion-paircapped quantum dots exhibit high external quantum efficiencies compared with the untreated QDs.

Original language	English (US)
Pages (from-to)	8718-8725
Number of pages	8
Journal	Advanced Materials
Volume	28
Issue number	39
DOIs	https://doi.org/10.1002/adma.201600784
State	Published - Aug 16 2016

Bibliographical note

KAUST Repository Item: Exported on 2020-10-01
Acknowledged KAUST grant number(s): KUS-11-009-21, URF/1/2268-01-01
Acknowledgements: J.P., L.N.Q., and Y.Z. contributed equally to this work. This publication is based in part on Awards KUS-11-009-21 and URF/1/2268-01-01 made by King Abdullah University of Science and Technology (KAUST), by the Ontario Research Fund Research Excellence Program, and by the Natural Sciences and Engineering Research Council (NSERC) of Canada. L. N. Quan and D. H. Kim acknowledge the financial support by the National Research Foundation of Korea Grant funded by the Korean Government (Grant No. 2014R1A2A1A09005656). The authors acknowledge Mrs. Nini Wei and Dr. Jun Li for TEM cross-sections.

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Pan, J., Quan, L. N., Zhao, Y., Peng, W., Banavoth, M., Sarmah, S. P., Yuan, M., Sinatra, L., AlYami, N. M., Liu, J., Yassitepe, E., Yang, Z., Voznyy, O., Comin, R., Hedhili, M. N., Mohammed, O. F., Lu, Z. H., Kim, D. H., Sargent, E. H., & Bakr, O. (2016). Highly Efficient Perovskite-Quantum-Dot Light-Emitting Diodes by Surface Engineering. Advanced Materials, 28(39), 8718-8725. https://doi.org/10.1002/adma.201600784

@article{401f02145c0d4fffbd56b5428ce40c60,

title = "Highly Efficient Perovskite-Quantum-Dot Light-Emitting Diodes by Surface Engineering",

abstract = "A two-step ligand-exchange strategy is developed, in which the long-carbon-chain ligands on all-inorganic perovskite (CsPbX3, X = Br, Cl) quantum dots (QDs) are replaced with halide-ion-pair ligands. Green and blue light-emitting diodes made from the halide-ion-paircapped quantum dots exhibit high external quantum efficiencies compared with the untreated QDs.",

author = "Jun Pan and Quan, {Li Na} and Yongbiao Zhao and Wei Peng and Murali Banavoth and Sarmah, {Smritakshi P.} and Mingjian Yuan and Lutfan Sinatra and AlYami, {Noktan Mohammed} and Jiakai Liu and Emre Yassitepe and Zhenyu Yang and Oleksandr Voznyy and Riccardo Comin and Hedhili, {Mohamed N.} and Mohammed, {Omar F.} and Lu, {Zheng Hong} and Kim, {Dong Ha} and Sargent, {Edward H.} and Osman Bakr",

note = "KAUST Repository Item: Exported on 2020-10-01 Acknowledged KAUST grant number(s): KUS-11-009-21, URF/1/2268-01-01 Acknowledgements: J.P., L.N.Q., and Y.Z. contributed equally to this work. This publication is based in part on Awards KUS-11-009-21 and URF/1/2268-01-01 made by King Abdullah University of Science and Technology (KAUST), by the Ontario Research Fund Research Excellence Program, and by the Natural Sciences and Engineering Research Council (NSERC) of Canada. L. N. Quan and D. H. Kim acknowledge the financial support by the National Research Foundation of Korea Grant funded by the Korean Government (Grant No. 2014R1A2A1A09005656). The authors acknowledge Mrs. Nini Wei and Dr. Jun Li for TEM cross-sections.",

year = "2016",

month = aug,

day = "16",

doi = "10.1002/adma.201600784",

language = "English (US)",

volume = "28",

pages = "8718--8725",

journal = "Advanced Materials",

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Pan, J, Quan, LN, Zhao, Y, Peng, W, Banavoth, M, Sarmah, SP, Yuan, M, Sinatra, L, AlYami, NM, Liu, J, Yassitepe, E, Yang, Z, Voznyy, O, Comin, R, Hedhili, MN , Mohammed, OF, Lu, ZH, Kim, DH, Sargent, EH & Bakr, O 2016, 'Highly Efficient Perovskite-Quantum-Dot Light-Emitting Diodes by Surface Engineering', Advanced Materials, vol. 28, no. 39, pp. 8718-8725. https://doi.org/10.1002/adma.201600784

TY - JOUR

T1 - Highly Efficient Perovskite-Quantum-Dot Light-Emitting Diodes by Surface Engineering

AU - Pan, Jun

AU - Quan, Li Na

AU - Zhao, Yongbiao

AU - Peng, Wei

AU - Banavoth, Murali

AU - Sarmah, Smritakshi P.

AU - Yuan, Mingjian

AU - Sinatra, Lutfan

AU - AlYami, Noktan Mohammed

AU - Liu, Jiakai

AU - Yassitepe, Emre

AU - Yang, Zhenyu

AU - Voznyy, Oleksandr

AU - Comin, Riccardo

AU - Hedhili, Mohamed N.

AU - Mohammed, Omar F.

AU - Lu, Zheng Hong

AU - Kim, Dong Ha

AU - Sargent, Edward H.

AU - Bakr, Osman

N1 - KAUST Repository Item: Exported on 2020-10-01 Acknowledged KAUST grant number(s): KUS-11-009-21, URF/1/2268-01-01 Acknowledgements: J.P., L.N.Q., and Y.Z. contributed equally to this work. This publication is based in part on Awards KUS-11-009-21 and URF/1/2268-01-01 made by King Abdullah University of Science and Technology (KAUST), by the Ontario Research Fund Research Excellence Program, and by the Natural Sciences and Engineering Research Council (NSERC) of Canada. L. N. Quan and D. H. Kim acknowledge the financial support by the National Research Foundation of Korea Grant funded by the Korean Government (Grant No. 2014R1A2A1A09005656). The authors acknowledge Mrs. Nini Wei and Dr. Jun Li for TEM cross-sections.

PY - 2016/8/16

Y1 - 2016/8/16

N2 - A two-step ligand-exchange strategy is developed, in which the long-carbon-chain ligands on all-inorganic perovskite (CsPbX3, X = Br, Cl) quantum dots (QDs) are replaced with halide-ion-pair ligands. Green and blue light-emitting diodes made from the halide-ion-paircapped quantum dots exhibit high external quantum efficiencies compared with the untreated QDs.

AB - A two-step ligand-exchange strategy is developed, in which the long-carbon-chain ligands on all-inorganic perovskite (CsPbX3, X = Br, Cl) quantum dots (QDs) are replaced with halide-ion-pair ligands. Green and blue light-emitting diodes made from the halide-ion-paircapped quantum dots exhibit high external quantum efficiencies compared with the untreated QDs.

UR - http://hdl.handle.net/10754/622107

UR - http://onlinelibrary.wiley.com/doi/10.1002/adma.201600784/abstract

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DO - 10.1002/adma.201600784

M3 - Article

C2 - 27529532

SN - 0935-9648

VL - 28

SP - 8718

EP - 8725

JO - Advanced Materials

JF - Advanced Materials

IS - 39

ER -

Highly Efficient Perovskite-Quantum-Dot Light-Emitting Diodes by Surface Engineering

Abstract

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