High-Performance Perovskite Single-Junction and Textured Perovskite/Silicon Tandem Solar Cells via Slot-Die Coating

Anand Selvin Subbiah; Furkan Halis Isikgor; Calvyn Travis Howells; Michele de Bastiani; Jiang Liu; Erkan Aydin; Francesco Furlan; Thomas Allen; Fuzong Xu; Shynggys Zhumagali; Sjoerd Hoogland; Edward H. Sargent; Iain McCulloch; Stefaan De Wolf

doi:10.1021/acsenergylett.0c01297

High-Performance Perovskite Single-Junction and Textured Perovskite/Silicon Tandem Solar Cells via Slot-Die Coating

Anand Selvin Subbiah, Furkan Halis Isikgor, Calvyn Travis Howells, Michele de Bastiani, Jiang Liu, Erkan Aydin, Francesco Furlan, Thomas Allen, Fuzong Xu, Shynggys Zhumagali, Sjoerd Hoogland, Edward H. Sargent, Iain McCulloch, Stefaan De Wolf

Research output: Contribution to journal › Article › peer-review

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Abstract

In this work we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent free, low-temperature (70 oC) slot-die coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic PTAA surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.

Original language	English (US)
Journal	ACS Energy Letters
DOIs	https://doi.org/10.1021/acsenergylett.0c01297
State	Published - Aug 11 2020

Bibliographical note

KAUST Repository Item: Exported on 2020-10-01
Acknowledgements: The authors acknowledge the support of the King Abdullah University of Science and Technology (KAUST) Office of Sponsored Research (OSR) under award no. KAUST OSR-CARF URF/1/3097, as well as funding support from QD Solar, Inc. The authors also thank the members of the KAUST Solar Center operations team for their valuable support. The authors also thank all the previous reports tabulated in Table S5 for the data points compiled in the TOC graphic

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10.1021/acsenergylett.0c01297

https://repository.kaust.edu.sa/bitstream/10754/664695/1/HHHigh%20performance.pdf

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Subbiah, A. S., Isikgor, F. H., Howells, C. T., de Bastiani, M., Liu, J., Aydin, E., Furlan, F., Allen, T., Xu, F., Zhumagali, S., Hoogland, S., Sargent, E. H., McCulloch, I., & De Wolf, S. (2020). High-Performance Perovskite Single-Junction and Textured Perovskite/Silicon Tandem Solar Cells via Slot-Die Coating. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.0c01297

@article{63131b7325754847ac6d58de1e383535,

title = "High-Performance Perovskite Single-Junction and Textured Perovskite/Silicon Tandem Solar Cells via Slot-Die Coating",

abstract = "In this work we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent free, low-temperature (70 oC) slot-die coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic PTAA surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.",

author = "Subbiah, {Anand Selvin} and Isikgor, {Furkan Halis} and Howells, {Calvyn Travis} and {de Bastiani}, Michele and Jiang Liu and Erkan Aydin and Francesco Furlan and Thomas Allen and Fuzong Xu and Shynggys Zhumagali and Sjoerd Hoogland and Sargent, {Edward H.} and Iain McCulloch and {De Wolf}, Stefaan",

note = "KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: The authors acknowledge the support of the King Abdullah University of Science and Technology (KAUST) Office of Sponsored Research (OSR) under award no. KAUST OSR-CARF URF/1/3097, as well as funding support from QD Solar, Inc. The authors also thank the members of the KAUST Solar Center operations team for their valuable support. The authors also thank all the previous reports tabulated in Table S5 for the data points compiled in the TOC graphic",

year = "2020",

month = aug,

day = "11",

doi = "10.1021/acsenergylett.0c01297",

language = "English (US)",

journal = "ACS Energy Letters",

issn = "2380-8195",

publisher = "American Chemical Society",

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AU - Subbiah, Anand Selvin

AU - Isikgor, Furkan Halis

AU - Howells, Calvyn Travis

AU - de Bastiani, Michele

AU - Liu, Jiang

AU - Aydin, Erkan

AU - Furlan, Francesco

AU - Allen, Thomas

AU - Xu, Fuzong

AU - Zhumagali, Shynggys

AU - Hoogland, Sjoerd

AU - Sargent, Edward H.

AU - McCulloch, Iain

AU - De Wolf, Stefaan

N1 - KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: The authors acknowledge the support of the King Abdullah University of Science and Technology (KAUST) Office of Sponsored Research (OSR) under award no. KAUST OSR-CARF URF/1/3097, as well as funding support from QD Solar, Inc. The authors also thank the members of the KAUST Solar Center operations team for their valuable support. The authors also thank all the previous reports tabulated in Table S5 for the data points compiled in the TOC graphic

PY - 2020/8/11

Y1 - 2020/8/11

N2 - In this work we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent free, low-temperature (70 oC) slot-die coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic PTAA surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.

AB - In this work we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent free, low-temperature (70 oC) slot-die coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic PTAA surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.

UR - http://hdl.handle.net/10754/664695

UR - https://pubs.acs.org/doi/10.1021/acsenergylett.0c01297

U2 - 10.1021/acsenergylett.0c01297

DO - 10.1021/acsenergylett.0c01297

M3 - Article

SN - 2380-8195

JO - ACS Energy Letters

JF - ACS Energy Letters

ER -

High-Performance Perovskite Single-Junction and Textured Perovskite/Silicon Tandem Solar Cells via Slot-Die Coating

Abstract

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