Environmental scanning ultrafast electron microscopy: Structural dynamics of solvation at interfaces

Ding Shyue Yang; Omar F. Mohammed; Ahmed H. Zewail

doi:10.1002/anie.201205093

Environmental scanning ultrafast electron microscopy: Structural dynamics of solvation at interfaces

Ding Shyue Yang, Omar F. Mohammed, Ahmed H. Zewail^*

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

24 Scopus citations

Abstract

On the surface: CdSe surfaces have been used as a prototype for the investigation of the spatiotemporal characteristics of solvation by environmental scanning ultrafast electron microscopy (see picture, GSED=gaseous secondary electron detector). This study has shown that the ultrafast relaxation dynamics of polar molecules, such as water, in the adsorbate layers exhibit a striking dependence on the CdSe surface structure.

Original language	English (US)
Pages (from-to)	2897-2901
Number of pages	5
Journal	Angewandte Chemie - International Edition
Volume	52
Issue number	10
DOIs	https://doi.org/10.1002/anie.201205093
State	Published - Mar 4 2013

Keywords

femtochemistry
microscopy
non-equilibrium processes
solvation
surface analysis

ASJC Scopus subject areas

General Chemistry
Catalysis

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abstract = "On the surface: CdSe surfaces have been used as a prototype for the investigation of the spatiotemporal characteristics of solvation by environmental scanning ultrafast electron microscopy (see picture, GSED=gaseous secondary electron detector). This study has shown that the ultrafast relaxation dynamics of polar molecules, such as water, in the adsorbate layers exhibit a striking dependence on the CdSe surface structure.",

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author = "Yang, {Ding Shyue} and Mohammed, {Omar F.} and Zewail, {Ahmed H.}",

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AU - Mohammed, Omar F.

AU - Zewail, Ahmed H.

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AB - On the surface: CdSe surfaces have been used as a prototype for the investigation of the spatiotemporal characteristics of solvation by environmental scanning ultrafast electron microscopy (see picture, GSED=gaseous secondary electron detector). This study has shown that the ultrafast relaxation dynamics of polar molecules, such as water, in the adsorbate layers exhibit a striking dependence on the CdSe surface structure.

KW - femtochemistry

KW - microscopy

KW - non-equilibrium processes

KW - solvation

KW - surface analysis

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Environmental scanning ultrafast electron microscopy: Structural dynamics of solvation at interfaces

Abstract

Keywords

ASJC Scopus subject areas

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