Electrodeposition of Hole-Transport Layer on Methylammonium Lead Iodide Film: A Strategy To Assemble Perovskite Solar Cells

Gergely F. Samu; Rebecca A. Scheidt; Gary Zaiats; Prashant V. Kamat; Csaba Janáky

doi:10.1021/acs.chemmater.8b01521

Electrodeposition of Hole-Transport Layer on Methylammonium Lead Iodide Film: A Strategy To Assemble Perovskite Solar Cells

Gergely F. Samu, Rebecca A. Scheidt, Gary Zaiats, Prashant V. Kamat, Csaba Janáky

Research output: Contribution to journal › Article › peer-review

16 Scopus citations

Abstract

The emergence of organic–inorganic metal halide perovskites as active components in solar cells has sparked a great interest in the scientific community. A steep rise was witnessed in the power conversion efficiencies, which currently peaks at a certified value of 22.7%.(1) The attractiveness of these materials resides in their exceptional defect tolerance,(2,3) tunable light absorption and emission properties,(4,5) enhanced charge carrier transport and lifetime,(4) and cost-effective preparation and processability.(6) Applications beyond solar cells have also been studied, in light emitting diodes,(7,8) lasers,(8) photodetectors,(9,10) X-ray detectors,(11) γ-detectors,(12) and smart windows.(13)

Original language	English (US)
Pages (from-to)	4202-4206
Number of pages	5
Journal	Chemistry of Materials
Volume	30
Issue number	13
DOIs	https://doi.org/10.1021/acs.chemmater.8b01521
State	Published - Jun 12 2018
Externally published	Yes

Bibliographical note

KAUST Repository Item: Exported on 2021-04-13
Acknowledged KAUST grant number(s): OCRF-2014-CRG3-2268
Acknowledgements: The authors thank Dr. Gabor London (Univ Szeged) for ́ synthesizing the bis-EDOT monomer as well as Dr. Tatyana Orlova and the Notre Dame Integrated Imaging Facility for taking the SEM images. This project has received funding from the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation program (grant agreement no. 716539). ELI-ALPS is supported by the
European Union and cofinanced by the European Regional Development Fund (GOP-1.1.1-12/B-2012-000, GINOP2.3.6-15-2015-00001). P.V.K. acknowledges support by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy (award DE-FC02-04ER15533). R.S. acknowledges support of King Abdullah University of Science and Technology (KAUST-Award OCRF-2014-CRG3-2268).
This publication acknowledges KAUST support, but has no KAUST affiliated authors.

ASJC Scopus subject areas

Materials Chemistry
General Chemical Engineering
General Chemistry

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10.1021/acs.chemmater.8b01521

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title = "Electrodeposition of Hole-Transport Layer on Methylammonium Lead Iodide Film: A Strategy To Assemble Perovskite Solar Cells",

abstract = "The emergence of organic–inorganic metal halide perovskites as active components in solar cells has sparked a great interest in the scientific community. A steep rise was witnessed in the power conversion efficiencies, which currently peaks at a certified value of 22.7%.(1) The attractiveness of these materials resides in their exceptional defect tolerance,(2,3) tunable light absorption and emission properties,(4,5) enhanced charge carrier transport and lifetime,(4) and cost-effective preparation and processability.(6) Applications beyond solar cells have also been studied, in light emitting diodes,(7,8) lasers,(8) photodetectors,(9,10) X-ray detectors,(11) γ-detectors,(12) and smart windows.(13)",

author = "Samu, {Gergely F.} and Scheidt, {Rebecca A.} and Gary Zaiats and Kamat, {Prashant V.} and Csaba Jan{\'a}ky",

note = "KAUST Repository Item: Exported on 2021-04-13 Acknowledged KAUST grant number(s): OCRF-2014-CRG3-2268 Acknowledgements: The authors thank Dr. Gabor London (Univ Szeged) for{\' } synthesizing the bis-EDOT monomer as well as Dr. Tatyana Orlova and the Notre Dame Integrated Imaging Facility for taking the SEM images. This project has received funding from the European Research Council (ERC) under the European Union{\textquoteright}s Horizon 2020 research and innovation program (grant agreement no. 716539). ELI-ALPS is supported by the European Union and cofinanced by the European Regional Development Fund (GOP-1.1.1-12/B-2012-000, GINOP2.3.6-15-2015-00001). P.V.K. acknowledges support by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy (award DE-FC02-04ER15533). R.S. acknowledges support of King Abdullah University of Science and Technology (KAUST-Award OCRF-2014-CRG3-2268). This publication acknowledges KAUST support, but has no KAUST affiliated authors.",

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doi = "10.1021/acs.chemmater.8b01521",

language = "English (US)",

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AU - Kamat, Prashant V.

AU - Janáky, Csaba

N1 - KAUST Repository Item: Exported on 2021-04-13 Acknowledged KAUST grant number(s): OCRF-2014-CRG3-2268 Acknowledgements: The authors thank Dr. Gabor London (Univ Szeged) for ́ synthesizing the bis-EDOT monomer as well as Dr. Tatyana Orlova and the Notre Dame Integrated Imaging Facility for taking the SEM images. This project has received funding from the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation program (grant agreement no. 716539). ELI-ALPS is supported by the European Union and cofinanced by the European Regional Development Fund (GOP-1.1.1-12/B-2012-000, GINOP2.3.6-15-2015-00001). P.V.K. acknowledges support by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy (award DE-FC02-04ER15533). R.S. acknowledges support of King Abdullah University of Science and Technology (KAUST-Award OCRF-2014-CRG3-2268). This publication acknowledges KAUST support, but has no KAUST affiliated authors.

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N2 - The emergence of organic–inorganic metal halide perovskites as active components in solar cells has sparked a great interest in the scientific community. A steep rise was witnessed in the power conversion efficiencies, which currently peaks at a certified value of 22.7%.(1) The attractiveness of these materials resides in their exceptional defect tolerance,(2,3) tunable light absorption and emission properties,(4,5) enhanced charge carrier transport and lifetime,(4) and cost-effective preparation and processability.(6) Applications beyond solar cells have also been studied, in light emitting diodes,(7,8) lasers,(8) photodetectors,(9,10) X-ray detectors,(11) γ-detectors,(12) and smart windows.(13)

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Electrodeposition of Hole-Transport Layer on Methylammonium Lead Iodide Film: A Strategy To Assemble Perovskite Solar Cells

Abstract

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