Depleted Bulk Heterojunction Colloidal Quantum Dot Photovoltaics

D. Aaron R. Barkhouse, Ratan Debnath, Illan J. Kramer, David Zhitomirsky, Andras G. Pattantyus-Abraham, Larissa Levina, Lioz Etgar, Michael Grätzel, Edward H. Sargent

Research output: Contribution to journalArticlepeer-review

216 Scopus citations

Abstract

The first solution-processed depleted bulk heterojunction colloidal quantum dot solar cells are presented. The architecture allows for high absorption with full depletion, thereby breaking the photon absorption/carrier extraction compromise inherent in planar devices. A record power conversion of 5.5% under simulated AM 1.5 illumination conditions is reported. Copyright © 2011 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Original languageEnglish (US)
Pages (from-to)3134-3138
Number of pages5
JournalAdvanced Materials
Volume23
Issue number28
DOIs
StatePublished - May 26 2011
Externally publishedYes

Bibliographical note

KAUST Repository Item: Exported on 2020-10-01
Acknowledged KAUST grant number(s): KUS-I1-009-21
Acknowledgements: D.A.R.B and R.D. contributed equally to this work. This publication is based on work supported in part by Award No. KUS-I1-009-21, made by King Abdullah University of Science and Technology (KAUST). The authors thank Angstrom Engineering and Innovative Technologies for useful discussions regarding material deposition methods and control of the glovebox environment, respectively. D.A.R.B. would like to thank the Ontario Postdoctoral Fellowship program and the Natural Sciences and Engineering Research Council for financial support. R.D. and I.J.K. acknowledge the financial support through e8/MITACS Elevate Strategic fellowship and the Queen Elizabeth II/Ricoh Canada Graduate Scholarship in Science and Technology, respectively. L.E. acknowledges the Marie Curie Actions-Intra-European Fellowships (FP7-PEOPLE-2009-IEF) under grant agreement no 252228. The authors would also like to acknowledge the technical assistance and scientific guidance of L. Brzozowski, E. Palmiano, R. Wolowiec, and D. Kopilovic.
This publication acknowledges KAUST support, but has no KAUST affiliated authors.

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