CO 2 Capture Capacity and Swelling Measurements of Liquid-like Nanoparticle Organic Hybrid Materials via Attenuated Total Reflectance Fourier Transform Infrared Spectroscopy

Youngjune Park; Dolly Shin; Young Nam Jang; Ah-Hyung Alissa Park

doi:10.1021/je200623b

CO 2 Capture Capacity and Swelling Measurements of Liquid-like Nanoparticle Organic Hybrid Materials via Attenuated Total Reflectance Fourier Transform Infrared Spectroscopy

Youngjune Park, Dolly Shin, Young Nam Jang, Ah-Hyung Alissa Park

Research output: Contribution to journal › Article › peer-review

50 Scopus citations

Abstract

Novel nanoparticle organic hybrid materials (NOHMs), which are comprised of organic oligomers or polymers tethered to an inorganic nanosized cores of various sizes, have been synthesized, and their solvating property for CO 2 was investigated using attenuated total reflectance (ATR) Fourier transform infrared (FT-IR) spectroscopy. Simultaneous measurements of CO 2 capture capacity and swelling behaviors of polyetheramine (Jeffamine M-2070) and its corresponding NOHMs (NOHM-I-PE2070) were reported at temperatures of (298, 308, 323 and 353) K and CO 2 pressure conditions ranging from (0 to 5.5) MPa. The polymeric canopy, or polymer bound to the nanoparticle surface, showed significantly less swelling behavior with enhanced or comparable CO 2 capture capacity compared to pure unbound polyetheramine. © 2011 American Chemical Society.

Original language	English (US)
Pages (from-to)	40-45
Number of pages	6
Journal	Journal of Chemical & Engineering Data
Volume	57
Issue number	1
DOIs	https://doi.org/10.1021/je200623b
State	Published - Oct 28 2011
Externally published	Yes

Bibliographical note

KAUST Repository Item: Exported on 2020-10-01
Acknowledged KAUST grant number(s): KUS-C1-018-02
Acknowledgements: This publication was based on work supported in part by Award No. KUS-C1-018-02, made by King Abdullah University of Science and Technology (KAUST), and the Utilization and Sequestration of CO2 using Industrial Minerals Program by Korea Institute of Geoscience & Mineral Resources (KIGAM).
This publication acknowledges KAUST support, but has no KAUST affiliated authors.

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10.1021/je200623b

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title = "CO 2 Capture Capacity and Swelling Measurements of Liquid-like Nanoparticle Organic Hybrid Materials via Attenuated Total Reflectance Fourier Transform Infrared Spectroscopy",

abstract = "Novel nanoparticle organic hybrid materials (NOHMs), which are comprised of organic oligomers or polymers tethered to an inorganic nanosized cores of various sizes, have been synthesized, and their solvating property for CO 2 was investigated using attenuated total reflectance (ATR) Fourier transform infrared (FT-IR) spectroscopy. Simultaneous measurements of CO 2 capture capacity and swelling behaviors of polyetheramine (Jeffamine M-2070) and its corresponding NOHMs (NOHM-I-PE2070) were reported at temperatures of (298, 308, 323 and 353) K and CO 2 pressure conditions ranging from (0 to 5.5) MPa. The polymeric canopy, or polymer bound to the nanoparticle surface, showed significantly less swelling behavior with enhanced or comparable CO 2 capture capacity compared to pure unbound polyetheramine. {\textcopyright} 2011 American Chemical Society.",

author = "Youngjune Park and Dolly Shin and Jang, {Young Nam} and Park, {Ah-Hyung Alissa}",

note = "KAUST Repository Item: Exported on 2020-10-01 Acknowledged KAUST grant number(s): KUS-C1-018-02 Acknowledgements: This publication was based on work supported in part by Award No. KUS-C1-018-02, made by King Abdullah University of Science and Technology (KAUST), and the Utilization and Sequestration of CO2 using Industrial Minerals Program by Korea Institute of Geoscience & Mineral Resources (KIGAM). This publication acknowledges KAUST support, but has no KAUST affiliated authors.",

year = "2011",

month = oct,

day = "28",

doi = "10.1021/je200623b",

language = "English (US)",

volume = "57",

pages = "40--45",

journal = "Journal of Chemical & Engineering Data",

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publisher = "American Chemical Society",

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CO 2 Capture Capacity and Swelling Measurements of Liquid-like Nanoparticle Organic Hybrid Materials via Attenuated Total Reflectance Fourier Transform Infrared Spectroscopy. / Park, Youngjune; Shin, Dolly; Jang, Young Nam et al.
In: Journal of Chemical & Engineering Data, Vol. 57, No. 1, 28.10.2011, p. 40-45.

Research output: Contribution to journal › Article › peer-review

TY - JOUR

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AU - Park, Youngjune

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AU - Jang, Young Nam

AU - Park, Ah-Hyung Alissa

N1 - KAUST Repository Item: Exported on 2020-10-01 Acknowledged KAUST grant number(s): KUS-C1-018-02 Acknowledgements: This publication was based on work supported in part by Award No. KUS-C1-018-02, made by King Abdullah University of Science and Technology (KAUST), and the Utilization and Sequestration of CO2 using Industrial Minerals Program by Korea Institute of Geoscience & Mineral Resources (KIGAM). This publication acknowledges KAUST support, but has no KAUST affiliated authors.

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AB - Novel nanoparticle organic hybrid materials (NOHMs), which are comprised of organic oligomers or polymers tethered to an inorganic nanosized cores of various sizes, have been synthesized, and their solvating property for CO 2 was investigated using attenuated total reflectance (ATR) Fourier transform infrared (FT-IR) spectroscopy. Simultaneous measurements of CO 2 capture capacity and swelling behaviors of polyetheramine (Jeffamine M-2070) and its corresponding NOHMs (NOHM-I-PE2070) were reported at temperatures of (298, 308, 323 and 353) K and CO 2 pressure conditions ranging from (0 to 5.5) MPa. The polymeric canopy, or polymer bound to the nanoparticle surface, showed significantly less swelling behavior with enhanced or comparable CO 2 capture capacity compared to pure unbound polyetheramine. © 2011 American Chemical Society.

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CO 2 Capture Capacity and Swelling Measurements of Liquid-like Nanoparticle Organic Hybrid Materials via Attenuated Total Reflectance Fourier Transform Infrared Spectroscopy

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