Allylic C(sp3)–H alkylation via synergistic organo- and photoredox catalyzed radical addition to imines

Jiaqi Jia; Rajesh Kancherla; Magnus Rueping; Long Huang

doi:10.1039/d0sc00819b

Allylic C(sp3)–H alkylation via synergistic organo- and photoredox catalyzed radical addition to imines

Jiaqi Jia, Rajesh Kancherla, Magnus Rueping, Long Huang

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Abstract

A new catalytic method for the direct alkylation of allylic C(sp$^{3}$)–H bonds from unactivated alkenes $\textit{via}$ synergistic organo- and photoredox catalysis is described.

Original language	English (US)
Pages (from-to)	4954-4959
Number of pages	6
Journal	Chemical Science
Volume	11
Issue number	19
DOIs	https://doi.org/10.1039/d0sc00819b
State	Published - Apr 30 2020

Bibliographical note

KAUST Repository Item: Exported on 2020-10-01
Acknowledgements: This work was financially supported by the King Abdullah University of Science and Technology (KAUST), Saudi Arabia, Office of Sponsored Research (URF/1/3754).

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10.1039/d0sc00819b

https://repository.kaust.edu.sa/bitstream/10754/662699/1/Articlefile1.pdf

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title = "Allylic C(sp3)–H alkylation via synergistic organo- and photoredox catalyzed radical addition to imines",

abstract = "A new catalytic method for the direct alkylation of allylic C(sp$^{3}$)–H bonds from unactivated alkenes $\textit{via}$ synergistic organo- and photoredox catalysis is described.",

author = "Jiaqi Jia and Rajesh Kancherla and Magnus Rueping and Long Huang",

note = "KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: This work was financially supported by the King Abdullah University of Science and Technology (KAUST), Saudi Arabia, Office of Sponsored Research (URF/1/3754).",

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AU - Jia, Jiaqi

AU - Kancherla, Rajesh

AU - Rueping, Magnus

AU - Huang, Long

N1 - KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: This work was financially supported by the King Abdullah University of Science and Technology (KAUST), Saudi Arabia, Office of Sponsored Research (URF/1/3754).

PY - 2020/4/30

Y1 - 2020/4/30

N2 - A new catalytic method for the direct alkylation of allylic C(sp$^{3}$)–H bonds from unactivated alkenes $\textit{via}$ synergistic organo- and photoredox catalysis is described.

AB - A new catalytic method for the direct alkylation of allylic C(sp$^{3}$)–H bonds from unactivated alkenes $\textit{via}$ synergistic organo- and photoredox catalysis is described.

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Allylic C(sp3)–H alkylation via synergistic organo- and photoredox catalyzed radical addition to imines

Abstract

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