A Rational Electrode-Electrolyte Design for Efficient Ammonia Electrosynthesis under Ambient Conditions

Bryan Harry Rahmat Suryanto, Colin Suk Mo Kang, Dabin Wang, Changlong Xiao, Fengling Zhou, Luis Azofra Mesa, Luigi Cavallo, Xinyi Zhang, Douglas R. Macfarlane

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214 Scopus citations

Abstract

Renewable energy driven ammonia electrosynthesis by N2 reduction reaction (NRR) at ambient conditions is vital for the sustainability of the global population and energy demand. However, NRR under ambient conditions to date has been plagued with low yield rate and selectivity (
Original languageEnglish (US)
Pages (from-to)1219-1224
Number of pages6
JournalACS Energy Letters
Volume3
Issue number6
DOIs
StatePublished - Apr 25 2018

Bibliographical note

KAUST Repository Item: Exported on 2020-10-01
Acknowledgements: The authors thank Monash Centre for Electron Microscopy (MCEM) for the provision of access to their instruments. L.M.A. and L.C. acknowledge King Abdullah University of Science and Technology (KAUST) for support. Gratitude is also due to the KAUST Supercomputing Laboratory using the supercomputer Shaheen II for providing the computational resources. This study was supported by an Australian Research Council (ARC) Discovery Grant (DP170102267). DRM is grateful to the ARC for his Australian Laureate Fellowship.

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